June 30, 2025 to July 4, 2025
Europe/Vienna timezone

Mutual Neutralization with initial-state control

Jul 3, 2025, 3:15 PM
1h 45m
Poster only Collisions of electrons, atoms, and molecules, highly charged ions, astrophysical processes Poster Session 3

Speaker

Henning T Schmidt (Stockholm University)

Description

The DESIREE double cryogenic storage ring at Stockholm University uniquely combines the ability to store and manipulate ions for extended periods of time with the merged-beams configuration allowing studies of sub-eV collisions between ions of opposite charges. By storage alone, molecules are allowed to relax vibrationally and rotationally towards their thermal equilibrium with the cryogenic surroundings, while in particular for small molecular and for atomic ions, the long storage time can be exploited to perform laser-manipulation. In this contribution we present four examples of experiments making use of this unique capability of DESIREE's.
Collision with oppositely charged fullerenes C$_{60}^+$ + C$_{60}^-$ [1], dissociate mutual neutralization in NO$^+$ + O$^-$ collisions [2], MN for metastable and ground state Si$^-$ with Na$^+$ and K$^+$ [3] and MN for Au$^-$ ions with Ba$^+$ with the initial state selected by optical pumping [4].

References
[1] M Gatchell et al. Astronomy & Astrophysics 693, A43 (2025).
[2] M Poline et al. Phys Rev Letters 132, 023001 (2024).
[3] R Poulose et al. To be submitted.
[4] R Poulose et al. To be submitted.

Authors

Rachel Poulose (Stockholm University) Paul Martini (Stockholm University, Stockholm, Sweden) Truly Rylander (Stockholm University) Sadiq Muhamed (Stockholm University) Mathias Poline (Stockholm University) Stefan Rosén (Stockholm University, Stockholm, Sweden) Ansgar Simonsson (Stockholm University) Michael Gatchell (Stockholm University, Stockholm, Sweden) Richard Thomas (Stockholm University) Henrik Cederquist (Stockholm University, Stockholm, Sweden) Dag Hanstorp (University of Gothenburg) Henning Zettergren (Stockholm University) Henning T Schmidt (Stockholm University)

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