June 30, 2025 to July 4, 2025
Europe/Vienna timezone

Spatially-resolved spin manipulation and readout of individual ultracold molecules in an optical lattice

Jul 1, 2025, 3:15 PM
1h 45m
Poster Cold and ultracold atoms, molecules and ions, degenerate quantum gases, ultracold plasmas Poster Session 2

Speaker

Benjamin Maddox (Durham University)

Description

Creating arrays of ultracold molecules for quantum simulation of many-body systems is rapidly becoming a reality [1,2]. A key requirement for high-fidelity simulation of various spin models is the ability to simultaneously recover the population in each spin state. Using a series of manipulations proposed in [3], we experimentally demonstrate that two rotational states of ultracold RbCs molecules can be mapped to their constituent atoms: a molecule in the upper (lower) rotational state is detected as a Cs (Rb) atom in our imaging. We load a 2D optical lattice with over a thousand molecules and, by projecting an addressing tweezer, imprint a localized spin impurity by shielding a region of the gas from microwave excitation to the upper rotational state. Using optical microscopy, we then spatially resolve this impurity with single-molecule resolution while simultaneously imaging the rest of the gas in the other spin state.

[1] - Cornish, S. L., Tarbutt, M. R., & Hazzard, K. R. (2024). Quantum computation and quantum simulation with ultracold molecules. Nature Physics, 20(5), 730-740.

[2]- Christakis, L., Rosenberg, J. S., Raj, R., Chi, S., Morningstar, A., Huse, D. A., ... & Bakr, W. S. (2023). Probing site-resolved correlations in a spin system of ultracold molecules. Nature, 614(7946), 64-69.

[3] - Covey, J. P., De Marco, L., Acevedo, Ó. L., Rey, A. M., & Ye, J. (2018). An approach to spin-resolved molecular gas microscopy. New Journal of Physics, 20(4), 043031.

Authors

Jonathan Mortlock (Durham University) Adarsh Raghuram (Durham University) Benjamin Maddox (Durham University) Philip Gregory (Durham University) Simon Cornish (Durham University)

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